{"id":11168,"date":"2026-08-26T21:37:29","date_gmt":"2026-08-26T13:37:29","guid":{"rendered":"\/jase\/?post_type=tkuisotope&#038;p=11168"},"modified":"2026-08-26T23:04:58","modified_gmt":"2026-08-26T15:04:58","slug":"jase-202612-35-004","status":"publish","type":"tkuisotope","link":"\/jase\/?tkuisotope=jase-202612-35-004","title":{"rendered":"Ozone-Regenerable Mesoporous Zeolite Y Pellets Synthesized Hydrothermally and Modified with Fe3+\/Mn2+ for Dye Adsorption"},"content":{"rendered":"\n<div class=\"wp-block-tkuwpbs5-bs5-row row article-info\">\n<div class=\"wp-block-tkuwpbs5-bs5-column col-md-3 align-self-start\">\n<p><i class=\"fa fa-folder\" aria-hidden=\"true\"><\/i>&nbsp;<a href=\"\/jase\/?page_id=807\" data-type=\"page\" data-id=\"807\">2026<\/a><\/p>\n<\/div>\n\n\n\n<div class=\"wp-block-tkuwpbs5-bs5-column col-md-3 align-self-start\">\n<p><i class=\"fa fa-folder-open\" aria-hidden=\"true\"><\/i>&nbsp;<a href=\"\/jase\/?page_id=11162\" data-type=\"page\" data-id=\"11162\">Volume 35<\/a><\/p>\n<\/div>\n\n\n\n<div class=\"wp-block-tkuwpbs5-bs5-column col-md-6 align-self-start\">\n<div class=\"wp-block-tkuwpbs5-bs5-div dv_publish\" data-aos=\"normal\"><div class=\"wp-block-post-date\"><time datetime=\"2026-08-26T21:37:29+08:00\">2026-08-26<\/time><\/div><\/div>\n<\/div>\n<\/div>\n\n\n\n<div class=\"wp-block-tkuwpbs5-bs5-row row\">\n<div class=\"wp-block-tkuwpbs5-bs5-column col-md-5 align-self-start\">\n<div class=\"wp-block-tkuwpbs5-bs5-div au-ol\" data-aos=\"normal\">\n<p>Vo Tran Minh Khoa<sup>1<\/sup>, Nguyen Manh Khang<sup>1<\/sup>, Huynh Diem Nhung<sup>1<\/sup>, Van Chi Khen<sup>1<\/sup>, Pham Thi Tuyet<sup>1,2<\/sup>, and Nguyen Quang Long<sup>1,2<\/sup><a href=\"mailto:nqlong@hcmut.edu.vn\"><i class=\"fa fa-envelope\"><\/i><\/a><\/p>\n\n\n\n<p style=\"font-size:14px\"><sup>1<\/sup>Faculty of Chemical Engineering, Ho Chi Minh City University of Technology (HCMUT), 268 Ly Thuong Kiet Street, Dien Hong <\/p>\n\n\n\n<p style=\"font-size:14px\"><sup>2<\/sup>ward, Ho Chi Minh City, Vietnam; Vietnam National University Ho Chi Minh City (VNU-HCM), Ho Chi Minh City, Vietnam<\/p>\n<\/div>\n\n\n\n<div class=\"wp-block-tkuwpbs5-bs5-div\" style=\"margin-top:var(--wp--preset--spacing--40)\" data-aos=\"normal\">\n<p>Received: March 30, 2026<br>Accepted: July 13, 2026<br>Publication Date: August 26, 2026<\/p>\n<\/div>\n<\/div>\n\n\n\n<div class=\"wp-block-tkuwpbs5-bs5-column col-md-7 align-self-start clk=\u5716\u7247\"><img decoding=\"async\" src=\"\/jase\/wp-content\/uploads\/2026\/08\/35_004.jpg\" class=\"img-fluid img-fluid mx-auto d-block\" alt=\"\u4e0a\u50b3\u5716\u7247\">\n\n\n<p class=\"has-text-align-center\">Column-based system design for methylene blue treatment.<\/p>\n<\/div>\n<\/div>\n\n\n\n<p class=\"has-small-font-size\"><i class=\"fab fa-creative-commons\"><\/i>&nbsp;<strong>Copyright&nbsp;<\/strong>The Author(s). This is an open access article distributed under the terms of the&nbsp;<a rel=\"noreferrer noopener\" href=\"https:\/\/creativecommons.org\/licenses\/by\/4.0\/\" target=\"_blank\">Creative Commons Attribution&nbsp;License (CC BY 4.0)<\/a>, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are cited.<\/p>\n\n\n\n<p>Download Citation:  <a href=\"\/jase\/wp-content\/uploads\/2026\/08\/V35.0004.txt\" data-type=\"attachment\" data-id=\"11218\" target=\"_blank\" rel=\"noreferrer noopener\">BibTeX <\/a>| <a rel=\"noreferrer noopener\" href=\"http:\/\/dx.doi.org\/10.6180\/jase.202612_35.004\" target=\"_blank\">http:\/\/dx.doi.org\/10.6180\/jase.202612_35.004<\/a>  <\/p>\n\n\n\n<p class=\"btn btn-primary article-btn\"><a href=\"\/jase\/wp-content\/uploads\/2026\/08\/004_2026_0672_V35.pdf\" data-type=\"attachment\" data-id=\"11179\" target=\"_blank\" rel=\"noreferrer noopener\">Download PDF<\/a><\/p>\n\n\n\n<div style=\"height:24px\" aria-hidden=\"true\" class=\"wp-block-spacer\"><\/div>\n\n\n\n<p>The design of regenerable adsorbents is critical for sustainable wastewater treatment. Mesoporous zeolite Y pellets were synthesized through hydrothermal dealumination-desilication and modified by Fe\u00b3\u207a and Mn\u00b2\u207a ion exchange. Characterization confirmed preservation of the FAU framework, while BET analysis showed enlarged external surface areas of 102 m\u00b2\/g for hierarchical Y, 81 m\u00b2\/g for VM80, and 72 m\u00b2\/g for Fe-VM80. Column experiments indicated that methylene blue adsorption followed pseudo-first-order kinetics[cite: 5]. Ozone regeneration outperformed the Fenton process, shortening treatment times to 1.5 h for Mn-VM80 and 1 h for Fe-VM80 while maintaining higher cyclic stability. The combination of hierarchical porosity, pelletization, and Fe\/Mn modification enabled efficient adsorption-desorption cycling. These ozone-regenerable mesoporous zeolite Y pellets show strong potential as scalable and sustainable adsorbents for dye removal.<\/p>\n\n\n\n<p><em>Keywords:&nbsp;Mesoporous zeolite Y; MB adsorption; Regeneration; Ozonation; hydrothermal synthesis<\/em><\/p>\n\n\n\n<div style=\"height:2rem\" aria-hidden=\"true\" class=\"wp-block-spacer\"><\/div>\n\n\n\n<div class=\"wp-block-tkuwpbs5-bs5-div ref_ol\" data-aos=\"normal\">\n<div class=\"container\">\n<div id=\"model-response-message-contentr_53180f64958e6cc2\" class=\"markdown markdown-main-panel md-content enable-luminous-fast-follows enable-updated-hr-color stronger\" dir=\"ltr\" aria-busy=\"false\" aria-live=\"polite\">\n<ol>\n<li data-path-to-node=\"0\">[1] D. Zhao, W. Zhang, C. Chen, and X. Wang, (2013) &#8220;Adsorption of Methyl Orange Dye Onto Multiwalled Carbon Nanotubes&#8221; Procedia Environmental Sciences 18: 890-895. DOI: 10.1016\/j.proenv.2013.04.120.<\/li>\n<li data-path-to-node=\"0\">[2] L. Wu, X. Liu, G. Lv, R. Zhu, L. Tian, M. Liu, Y. Li, W. Rao, T. Liu, and L. Liao, (2021) &#8220;Study on the adsorption properties of methyl orange by natural one-dimensional nano-mineral materials with different structures&#8221; Scientific Reports 11: 10640. DOI: 10.1038\/s41598-021-90235-1.<\/li>\n<li data-path-to-node=\"0\">[3] S. Rahmani, B. Zeynizadeh, and S. Karami, (2020) &#8220;Removal of cationic methylene blue dye using magnetic and anionic-cationic modified montmorillonite: kinetic, isotherm and thermodynamic studies&#8221; Applied Clay Science 184: 105391. DOI: 10.1016\/j.clay.2019.105391.<\/li>\n<li data-path-to-node=\"0\">[4] J. Fito, M. Abewaa, A. Mengistu, K. Angassa, A. D. Ambaye, W. Moyo, and T. Nkambule, (2023) &#8220;Adsorption of methylene blue from textile industrial wastewater using activated carbon developed from Rumex abyssinicus plant&#8221; Scientific Reports 13: 5427. DOI: 10.1038\/s41598-023-32341-w.<\/li>\n<li data-path-to-node=\"0\">[5] N. M. Thuan, N. T. M. Linh, N. T. T. Phuong, N. T. H. Duong, N. M. Hung, P. T. Tuyet, N. Van Dung, and N. Q. Long, (2024) &#8220;Ethanolamine-modified zeolite-Chitosan beads as new adsorbents for carbon dioxide capture and crystal violet removal&#8221; Case Studies in Chemical and Environmental Engineering 10: 100917. DOI: 10.1016\/j.cscee.2024.100917.<\/li>\n<li data-path-to-node=\"0\">[6] F. Poorsajadi, M. H. Sayadi, M. Hajiani, and M. R. Rezaei, (2022) &#8220;Synthesis of CuO\/Bi2O3 nanocomposite for efficient and recycling photodegradation of methylene blue dye&#8221; International Journal of Environmental Analytical Chemistry 102: 7165-7178. DOI: 10.1080\/03067319.2020.1826464.<\/li>\n<li data-path-to-node=\"0\">[7] C. Kathing and G. Saini, (2022) &#8220;A Review of Various Treatment Methods for the Removal of Dyes from Textile Effluent&#8221; Recent Progress in Materials 4: 1-15. DOI: 10.21926\/rpm.2204028.<\/li>\n<li data-path-to-node=\"0\">[8] C. Langa, N. Mabuba, L. M. Mahlaule-Glory, D. E. Motaung, Z. Tetana, and N. C. Hintsho-Mbita, (2026) &#8220;Enhanced photocatalytic degradation of dyes and pharmaceutical pollutants using Fe\/TiO2-carbon nanospheres from Sutherlandia Frutescence&#8221; International Journal of Environmental Analytical Chemistry 106: 790-820. DOI: 10.1080\/03067319.2025.2524833.<\/li>\n<li data-path-to-node=\"0\">[9] L. Mouni, L. Belkhiri, J.-C. Bollinger, A. Bouzaza, A. Assadi, A. Tirri, F. Dahmoune, K. Madani, and H. Remini, (2018) &#8220;Removal of Methylene Blue from aqueous solutions by adsorption on Kaolin: Kinetic and equilibrium studies&#8221; Applied Clay Science 153: 38-45. DOI: 10.1016\/j.clay.2017.11.034.<\/li>\n<li data-path-to-node=\"0\">[10] G. Bal and A. Thakur, (2022) &#8220;Distinct approaches of removal of dyes from wastewater: A review&#8221; Materials Today: Proceedings 50: 1575-1579. DOI: 10.1016\/j.matpr.2021.09.119.<\/li>\n<li data-path-to-node=\"0\">[11] K. Rida, S. Bouraoui, and S. Hadnine, (2013) &#8220;Adsorption of methylene blue from aqueous solution by kaolin and zeolite&#8221; Applied Clay Science 83-84: 99-105. DOI: 10.1016\/j.clay.2013.08.015.<\/li>\n<li data-path-to-node=\"0\">[12] T. P. Le, H. V. T. Luong, H. N. Nguyen, T. K. T. Pham, T. L. Trinh Le, T. B. Q. Tran, and T. N. M. Ngo, (2024) &#8220;Insight into adsorption-desorption of methylene blue in water using zeolite NaY: Kinetic, isotherm and thermodynamic approaches&#8221; Results in Surfaces and Interfaces 16: 100281. DOI: 10.1016\/j.rsurfi.2024.100281.<\/li>\n<li data-path-to-node=\"0\">[13] N. M. Khang, V. T. Minh Khoa, N. T. Truc Phuong, N. X. Du, N. T. Hoang Duong, N. Van Dung, T. T. Tuyet Mai, and N. Q. Long, (2025) &#8220;Double-xerogel network composite zeolite granules targeting dual-functional fertilizers&#8221; Case Studies in Chemical and Environmental Engineering 12: 101253. DOI: 10.1016\/j.cscee.2025.101253.<\/li>\n<li data-path-to-node=\"0\">[14] D. M. El-Mekkawi, F. A. 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DOI: 10.1007\/s11356-016-6835-6.<\/li>\n<\/ol>\n<\/div>\n<\/div>\n<\/div>\n\n\n\n<p><\/p>\n","protected":false},"author":3,"template":"wp-custom-template-detail-4-aricles","meta":{"_uag_custom_page_level_css":""},"categories":[12,1956,6],"tags":[1960],"acf":[],"uagb_featured_image_src":[],"uagb_author_info":{"display_name":"\u6797\u923a\u6db5","author_link":"\/jase\/?author=3"},"uagb_comment_info":0,"uagb_excerpt":"&nbsp;Copyright&nbsp;The Author(s). This is an open access article distributed under the terms of the&nbsp;Creative Commons Attribution&nbsp;License (CC BY 4.0), which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are cited. Download Citation: BibTeX | http:\/\/dx.doi.org\/10.6180\/jase.202612_35.004 Download PDF The design of regenerable adsorbents is critical for sustainable wastewater treatment.&hellip;","_links":{"self":[{"href":"\/jase\/index.php?rest_route=\/wp\/v2\/tkuisotope\/11168"}],"collection":[{"href":"\/jase\/index.php?rest_route=\/wp\/v2\/tkuisotope"}],"about":[{"href":"\/jase\/index.php?rest_route=\/wp\/v2\/types\/tkuisotope"}],"author":[{"embeddable":true,"href":"\/jase\/index.php?rest_route=\/wp\/v2\/users\/3"}],"wp:attachment":[{"href":"\/jase\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=11168"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/jase\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=11168"},{"taxonomy":"post_tag","embeddable":true,"href":"\/jase\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=11168"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}